The activity of catalyst was improved with increasing CeO_2 content. The addition of CeO_2 was benefit to Cu dispersion and influence the distribution of Cu species on catalyst surface. Cu~+ could be stabilized in Ce-Zr-O lattice.

 
  • 对催化剂中CeO_2含量的影响进行了研究,催化剂活性随CeO_2含量增大而升高,TPR和XPS分析发现,催化剂中CeO_2含量增大,有利于增大Cu在载体表面的分散度,添加CeO_2之后催化剂表面出现Cu~+,Cu的多价态特性增强了Ce的Redox能力;
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